Planckian dissipation, anomalous high temperature THz non-linear response and energy relaxation in the strange metal state of the cuprate superconductors

We have investigated the nonlinear THz 2D coherent spectroscopic response of superconducting La_2−xSr_xCuO₄ (LSCO) thin films as a function of T across a wide range of doping levels from mildly underdoped through extremely overdoped (Tc<5 K). In addition to the large nonlinearities expected in the superconducting state, we find an extended regime of large normal state THz nonlinearity. This is in sharp contrast to the conventional superconductor NbN where the strong nonlinear response promptly disappears at Tc. The size of the nonlinear susceptibility in LSCO is |χ(3)|≈2.2×10−9m²/V², which is one of the largest THz range nonlinearities ever measured. The 2DCS measurement shows that the dominant normal state nonlinearities arise from pump-probe processes, of which there are various possible origins. These may be related to the unconventional interactions that lead to the strange metal or the persistence of superconducting correlations to high temperatures. Irrespective of its origin, the large normal state nonlinearity provides an opportunity to measure the energy relaxation rate (ΓE) to temperatures where the momentum relaxation rate is linear in T and close to its ``Planckian" form (Γ_M≈2kT/h). We find Γ_E to be 10−40 times smaller than the momentum relaxation. This shows that the scattering that causes momentum loss (and T-linear) resistivity do not remove appreciable energy from the electrons. Although the T-dependence of the momentum relaxation is consistent with quasi-elastic scattering off bosonic collective modes at temperatures above their characteristic energy (the Bloch-Gruneisen temperature for acoustic phonons) it is inconsistent with Γ_E's temperature dependence. Γ_E is an increasing function of T, which is indicative of inelastic scattering to the phonon bath.