Imaging twisted bilayer 1T’-WTe<sub>2</sub> with scanning tunneling microscopy and spectroscopy

ORAL

Abstract

Moiré patterns in two-dimensional materials arise from interference between lattices with a small lattice-constant mismatch or a slight rotational misalignment, offering means to engineer emergent structural and electronic phenomena. Twisted bilayer 1T’-WTe2 (tWTe2) is a notable example. In monolayer form, WTe2 is a candidate topological excitonic insulator at charge neutrality and becomes superconducting upon electron doping. When two layers are twisted slightly away from the natural bilayer stacking, tWTe2 is expected to form a rectangular moiré pattern. This texture hosts domains of alternating out-of-plane ferroelectric polarization separated by one-dimensional solitonic domain walls, with potential connections to coupled-wire Luttinger liquid models. Despite these prospects, experimental studies of tWTe2 remain limited, in part due to fabrication challenges. Here, we report scanning tunneling microscopy and spectroscopy (STM/S) of small-angle tWTe2, enabled by recent advances in device assembly. We identify solitonic domain walls in STM topography and investigate their structural and electronic properties under electrostatic gating. Our results establish tWTe2 as a promising platform for one-dimensional physics, and open a path to systematic twist-angle-dependent studies.

Presenters

  • Keng Tou Chu

    • University of Washington

Authors

  • Keng Tou Chu

    • University of Washington
  • Florie Mesple

    • University of Washington
  • Ellis Thompson

    • University of Washington
  • Jackson Chapman

    • University of Washington
  • Chaowei Hu

    • University of California, Los Angeles
    • University of Washington
  • Kenji Watanabe

    • National Institute for Materials Science
    • Research Center for Functional Materials, National Institute of Materials Science, 1-1 Namiki Tsukuba, Ibaraki 305-0044, Japan
  • Takashi Taniguchi

    • National Institute for Materials Science
    • Research Center for Materials Nanoarchitectonics, National Institute for Materials Science
    • International Center for Materials Nanoarchitectonics, National Institute of Materials Science, 1-1 Namiki Tsukuba, Ibaraki 305-0044, Japan
    • Research Center for Functional Materials, National Institute of Materials Science, 1-1 Namiki Tsukuba, Ibaraki 305-0044, Japan
  • Xiaodong Xu

    • University of Washington
  • David Cobden

    • University of Washington
  • Jiun-Haw Chu

    • University of Washington
  • Matthew A Yankowitz

    • University of Washington