Intertwined Short-Range Charge Correlations and Superconductivity in Sn-doped CsV<sub>3</sub>Sb<sub>5</sub>

ORAL

Abstract

The kagome metal CsV3Sb5 provides a unique platform to study the interplay between charge density wave (CDW) order and superconductivity. Hole doping via Sn substitution tunes the band filling, suppressing CDW formation and enhancing superconductivity in a characteristic double-dome phase diagram. We present a comprehensive investigation of charge correlations across the Sn-doped CsV3Sb5 series and their connection to the superconducting state. At low doping, the long-range 2 × 2 × 4 CDW order and associated superconducting fluctuations of the parent compound are rapidly suppressed. With further doping, the 2 × 2 × 2 CDW phase vanishes, giving rise to short-range quasi-1D correlations that persist throughout the second superconducting dome. As TC decreases at higher doping, these correlations fade, suggesting that superconductivity in this regime relies on short-range charge order. We further propose a V-V dimer formation model within the kagome plane to describe these short-range correlations, where local rotational and translational symmetry breaking may play a key role in stabilizing the second superconducting dome.

*This research was supported by the UC Santa Barbara NSF Quantum Foundry funded via the Q-AMASE-i program under award DMR-1906325. We acknowledge the use of shared facilities of the NSF MRSEC at UC Santa Barbara [DMR 1720256] and the Center for Scientific Computing, supported by the California Nano Systems Institute, the NSF MRSEC [DMR 1720256] and NSF CNS 1725797. The MRL Shared Experimental Facilities are supported by the MRSEC Program of the NSF under Award No. DMR 2308708; a member of the NSF-funded Materials Research Facilities Network (www.mrfn.org). Research conducted at the Center for High-Energy X-ray Science (CHEXS) is supported by the NSF (BIO, ENG and MPS Directorates) under award DMR-1829070 and DMR-2342336. Work by B.R.O. was supported by the U.S. Department of Energy (DOE), Office of Science, Basic Energy Sciences (BES), Materials Sciences and Engineering Division.

Presenters

  • Andrea Nataly Capa Salinas

    • University of California, Santa Barbara

Authors

  • Andrea Nataly Capa Salinas

    • University of California, Santa Barbara
  • Brenden R Ortiz

    • Oak Ridge National Laboratory
  • Steven J Gomez Alvarado

    • University of California, Santa Barbara
    • Rice University
  • Sarah A Schwarz

    • University of California, Santa Barbara
  • Ganesh Pokharel

    • University of California, Santa Barbara
    • University of West Georgia
  • Shiyu Yuan

    • UC Santa Barbara
  • Roland Yin

    • University of California, Santa Barbara
  • Suchismita Sarker

    • CHESS
  • Stephen Wilson

    • University of California, Santa Barbara