Signatures of unconventional pairing and gapless superconductivity in the kagome superconductors Cs(V<sub>1-x</sub>Ti<sub>x</sub>)<sub>3</sub>Sb<sub>5</sub>

ORAL

Abstract

Although the recently discovered vanadium-based kagome superconductors AV₃Sb₅ (A = K, Rb, and Cs) are promising candidates for hosting unconventional superconductivity, the true nature of their superconducting gaps remains elusive. Here, we report temperature- and magnetic-field-dependent thermal conductivity (κ) measurements on Ti-substituted Cs(V₁₋ₓTiₓ)₃Sb₅ (x = 0.0–0.06). For samples within the first superconducting dome (0.0 ≤ x ≤ 0.02), κ(T) revealed excitations consistent with a small full gap and a monotonic suppression of the gap minimum with increasing x. In the same range, κ(H) showed that quasiparticles were easily excited and delocalized by small fields along the c axis, resembling the behavior of nodal superconductors. Moreover, the electronic κ approached its normal-state value well below Hc2, uncovering an anomalous gapless superconducting state. These results strongly support unconventional chiral d + id pairing in the first dome, characterized by a fragile full gap susceptible to time–reversal–symmetry–breaking perturbations.

*This project was financially supported by the Ministry of Science and ICT through the National Research Foundation of Korea (2022M3K2A1083855 and RS-2024-00338707) and by the Ministry of Education (2021R1A6C101B418).

Publication: K. Nam, et al., Signatures of unconventional pairing and gapless superconductivity in the kagome superconductors Cs(V1-xTix)3Sb5.
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Presenters

  • Kiwan Nam

    • Seoul National University

Authors

  • Kiwan Nam

    • Seoul National University
  • Kwang-Tak Kim

    • Seoul National University
  • Yeahan Sur

    • Seoul National University
  • Kee Hoon Kim

    • Seoul National University
  • Woo-Yong Kim

    • Daegu Gyeongbuk Institute of Science and Technology
  • Jungpil Seo

    • Daegu Gyeongbuk Institute of Science and Technology