Magnetic Phases in Ca$2$Ru${1-x}$Mn$_x$O$_4$

ORAL

Abstract

The evolution of magnetic order in \textbf{Ca$_2$Ru$_{1-x}$Mn$_x$O$_4$} ($x = 0.03$--$0.14$) has been investigated using neutron diffraction. Mn doping preserves the low-temperature orthorhombic symmetry (\textit{Pbca}) but weakens the orthorhombic distortion by reducing the difference between the $a$ and $b$ axes. It also systematically enhances the antiferromagnetic transition temperature and modifies the balance between two competing magnetic structures: the \textit{A}-centered and \textit{B}-centered phases. With increasing Mn content, the \textit{B}-centered phase progressively expands at the expense of the \textit{A}-centered one, which becomes short-ranged at $x = 0.14$. These results underscore the crucial role of orbital degrees of freedom in driving the magnetic phase competition in this layered ruthenate.

*This research used resources at the High Flux Isotope Reactor, a DOE Office of Science User Facility operated by the Oak Ridge National Laboratory.

Presenters

  • Songxue Chi

    • Oak Ridge National Laboratory

Authors

  • Songxue Chi

    • Oak Ridge National Laboratory
  • Feng Ye

    • Oak Ridge National Laboratory
  • Gang Cao

    • University of Colorado, Boulder