Localized Skyrmion Formation in Amorphous Fe<sub>0.56</sub> Ge<sub>0.44</sub> Thin Films Driven by Intrinsic Magnetic Disorder

ORAL

Abstract

Magnetic skyrmions are topologically protected spin textures stabilized by Dzyaloshinskii–Moriya interactions (DMI) under moderate magnetic fields and temperatures. Here, we report the emergence of skyrmion pockets in amorphous Fe0.56 Ge0.44 thin films at the boundaries of helical domains, revealing novel topological behavior in structurally disordered magnetic materials. Using Lorentz transmission electron microscopy (LTEM), we observe the spontaneous nucleation of non-collinear spin textures at 205 K, which collapse into stable Bloch skyrmions with diameters of approximately 80 nm under a modest applied field, similar to that seen in B20 phase except that here the skyrmions have approximately equal distribution of up and down chirality. The distribution of skyrmions is attributed to atomic-scale fluctuations in exchange, anisotropy, and DMI intrinsic to the glassy structure. Our findings demonstrate a new route to stabilize metastable topological textures through structural disorder, opening avenues for reconfigurable spintronic devices. This study expands the fundamental phase diagram of skyrmion hosts and suggests amorphous magnets as versatile platforms for robust, high-density information storage and neuromorphic computing.

*This work has been primarily supported by the U.S. DOE-BES through contract DE-AC02-05-CH11231 (NEMM FWP). Additional support for Lorentz TEM work was provided by the Molecular Foundry and was supported by the Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231.

Presenters

  • Subhashree Satapathy

    • Lawrence Berkeley National Laboratory

Authors

  • Subhashree Satapathy

    • Lawrence Berkeley National Laboratory
  • Reed Yalisove

    • University of California, Berkeley
  • Temuujin Bayaraa

    • Lawrence Berkeley National Laboratory
  • Sinéad M Griffin

    • Lawrence Berkeley National Laboratory
  • Sujoy Roy

    • Lawrence Berkeley National Laboratory
  • Peter Fischer

    • Lawrence Berkeley National Laboratory
  • Mary Scott

    • University of California, Berkeley
  • Frances Hellman

    • University of California,Berkeley
    • University of California, Berkeley