Interparticle interaction-dependent critical point(s) govern yielding in soft particulate systems
ORAL
Abstract
Soft particulate materials exhibit a solid–fluid transition under shear. In the non-inertial regime, yielding is generically a two-step transition process that organizes a universal rheology across these systems. Using natural Soft-Earth suspensions as a model system, we identify: (i) an elastic-to-plastic transition at a lower critical shear rate, where an amorphous solid deforms and initiates flow, and (ii) a plastic to viscous transition at a higher critical shear rate where hydrodynamic dissipation dominates and a high-shear Newtonian limit emerges. We classify particulate systems by dominant interactions at the constituent particle scale. Frictional (granular) systems concentrate the two transitions to a single critical point, producing Bingham-like behavior and abrupt failure akin to Coulomb friction. Non-frictional systems (colloids, emulsions, and gels) generically possess two distinct critical points and exhibit a mix of Bingham and Herschel-Bulkley type flow, where the effective exponent reflects the distance between critical points and the underlying interparticle interactions in the system. By unifying granular rheology with elastoplastic models, the grain-scale interaction dependent two-point critical picture provides predictive control of plastic yielding across soft matter, relevant to manufacturing, geophysical hazard prediction, and complex fluids design.
*NASA TRUSSES, NSF ERC for IoT4Ag, Penn Center for Soft and Living Matter Postdoc Fellowship
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Publication: 1. Shravan Pradeep, Paulo E. Arratia, Douglas J. Jerolmack, "Universal rheology framework for yielding soft particulate materials", In Preparation.
2. Shravan Pradeep, Paulo E. Arratia, Douglas J. Jerolmack, "Origins of complexity in Soft Earth suspensions", Nature Communications (2024).
3. Robert Kostynick*, Hadis Matinpour*, Shravan Pradeep*, Sarah Haber, Alban Sauret, Eckart Meiburg, Thomas Dunne, Paulo Arratia, Douglas Jerolmack, "Rheology of debris-flow materials is controlled by the distance from jamming", PNAS (2022). *equal contribution
Presenters
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Shravan Pradeep
- University of Pennsylvania