Mechanochemical feedback drives complex inertial dynamics in active solids

ORAL

Abstract

By combining internal driving (activity) with elasticity, active solid systems can exhibit nonequilibrium mechanics and autonomous motion. While these systems are often studied in overdamped settings, e.g., in soft materials, the role of inertia has received less attention. We propose a model of a chemically active solid that includes mechanochemical feedback. Our findings reveal that when this feedback dominates over mechanical damping, autonomous inertial dynamics can spontaneously emerge through the sustained consumption of chemical fuel. By integrating numerical simulations, analytical methods, and approaches from dynamical systems, we demonstrate how active feedback drives complex nonlinear dynamics across multiple time scales, including limit cycles and chaotic behavior. Our results suggest design principles for the development of ultrafast actuators and autonomous machines made from soft, chemically powered solids.

*N.B., X.M. and B.A. acknowledge support from the US Army Research Office (Grant No. W911NF-20-2-0182). X.M., S.S., and Y.W. acknowledge support from the Office of Naval Research (MURI N00014-20-1-2479). X.M. acknowledge support from National Science Foundation through the Materials Research Science and Engineering Center at the University of Michigan, Award No. DMR-2309029. This research was supported in part by grant NSF PHY-2309135 to the Kavli Institute for Theoretical Physics (KITP).

Publication: arXiv:2505.18272

Presenters

  • Biswarup Ash

    • University of Michigan- Ann Arbor

Authors

  • Biswarup Ash

    • University of Michigan- Ann Arbor
  • Siddhartha Sarkar

    • Max Planck Institute for the Physics of Complex Systems
  • Nicholas Boechler

    • University of California, San Diego
  • Yueyang Wu

    • University of Michigan
  • Suraj Shankar

    • University of Michigan
  • Xiaoming Mao

    • University of Michigan