Mapping the Moiré Potential in Multi-Layer Rhombohedral Graphene

ORAL

Abstract

Rhombohedral graphene (rG) aligned with hexagonal boron nitride (hBN) has been shown to host flat bands that stabilize various strongly correlated quantum phases, including Mott insulators, integer, and fractional quantum anomalous Hall phases. In this work, we use scanning tunneling microscopy/spectroscopy (STM/STS) to visualize the dispersion of flat bands with doping and applied displacement fields in a hBN-aligned rhombohedral trilayer graphene (rtG)/hBN moiré superlattice. In addition to the intrinsic flat bands of rtG induced by the displacement field, we observe low-energy features originating from moiré potential-induced band folding. Real-space variations of the spectroscopic features allow us to quantify the spatial structure of the moiré potential at the rtG/hBN interface. Importantly, we find that accurately capturing the moiré site-dependent spectra requires incorporating a moiré potential acting on the top graphene layer with a sign opposite to that of the bottom layer into the continuum model. Our results thus provide key experimental and theoretical insights into understanding the role of the moire superlattice in rG/hBN heterostructures.

*This work was supported by Programmable Quantum Materials, an Energy Frontier Research Center funded by the U.S. Department of Energy (DOE), Office of Science, Basic Energy Sciences (BES) under award no. DE-SC0019443. The Flatiron Institute is a division of the Simons Foundation.

Publication: https://arxiv.org/abs/2510.09548

Presenters

  • Eric Seewald

    • Columbia University

Authors

  • Eric Seewald

    • Columbia University
  • Sanat Ghosh

    • Columbia University
  • Nishchhal Verma

    • Columbia University
  • John Cenker

    • Columbia University
  • Yinan Dong

    • Columbia University
    • University of Chicago
  • Birui Yang

    • Columbia University
  • Amit Basu

    • Tata Institute of Fundamental Research
  • Takashi Taniguchi

    • National Institute for Materials Science
    • Research Center for Materials Nanoarchitectonics, National Institute for Materials Science
    • International Center for Materials Nanoarchitectonics, National Institute of Materials Science, 1-1 Namiki Tsukuba, Ibaraki 305-0044, Japan
    • Research Center for Functional Materials, National Institute of Materials Science, 1-1 Namiki Tsukuba, Ibaraki 305-0044, Japan
  • Kenji Watanabe

    • National Institute for Materials Science
    • Research Center for Functional Materials, National Institute of Materials Science, 1-1 Namiki Tsukuba, Ibaraki 305-0044, Japan
  • Mandar M Deshmukh

    • Tata Institute of Fundamental Research (TIFR)
  • Dimitri Basov

    • Columbia University
  • Raquel Queiroz

    • Department of Physics, Columbia University, New York, NY, USA
    • Columbia University
  • Cory R Dean

    • Columbia University
  • Abhay Pasupathy

    • Columbia University
    • Columbia University/Brookhaven National Laboratory