OPTICAL CONTROL OF VO<sub>2 </sub>HETEROSTRUCTURES

ORAL

Abstract

The condensed matter community has kept a growing interest in VO2 due to its key role in the realization of neuromorphic computing devices and other resistive-switching applications. Nevertheless, its strong insulator-to-metal transition (IMT) close to room temperature and the possibility to grow thin films in a simple sputtering chamber opens the door to the fabrication of heterostructures based in VO2 with expanded functionalities. In this work, we present a simple structure based on the combination of high quality VO2 thin films and optically active metallic nanostructures. We aim to understand the interplay between the optical and electrical response in the system while characterizing the thermal dynamics of the system. Often overlooked, the local temperature in the VO2 film can be greatly impacted by an external electric field or light in the visible and near-infrared regimes. By combining optical excitation, structural characterization, and thermal and transport measurements we are able to shed light in the complex interplay between electrical and optical degrees of freedom.

*Work supported by the Air Force Office of Scientific Research under award number FA9550-22-1-0135. This work was performed in part at the San Diego Nanotechnology Infrastructure (SDNI) of UCSD, a member of the National Nanotechnology Coordinated Infrastructure, which is supported by the National Science Foundation (Grant ECCS-2025752). Ministerio de Ciencia e Investigación and Agencia Estatal de Investigación through the grants CNS2023-144128 (A.M-N.), PID2024-157080OB-C31(A.M-N) and PID2024-157080OA-C33 (M.A) and RYC2022-035912-I (J.L-S.). AGM and BCLdL acknowledged funding from PID2022-137569NB-C41 (LIGHTCOMPAS), funded by MCIN/AEI/10.13039/501100011033, “ERDF A way of making Europe”, BCLdL acknowledges a predoctoral contract funded as well by “ESF Investing in your future” (PREP2022-000426).

Presenters

  • Javier Rodrigues Alvarez

    • University of California, San Diego
    • University of California San Diego

Authors

  • Javier Rodrigues Alvarez

    • University of California, San Diego
    • University of California San Diego
  • Álvaro Muñoz-Noval

    • Dpto. Física Materiales, Facultad CC. Físicas, Universidad Complutense de Madrid, Madrid, 28040 Spain
  • Juan A Hofer

    • University of California, San Diego
  • Manuel Abuin

    • e Instituto de Sistemas Optoelectrónicos y Microtecnología (ISOM-UPM), 28040 Madrid, Spain
  • Jesus Lopez-Sanchez

    • Departamento de Electrocerámica, Instituto de Cerámica y Vidrio, Consejo Superior de Investigaciones Científicas, Calle Kelsen 5, Madrid 28049, Spain
  • Beatriz Castillo Lopez de Larrinzar

    • Instituto de Micro y Nanotecnología IMN-CNM, CSIC, CEI UAM + CSIC, Isaac Newton 8, 28760, Tres Cantos, Madrid, Spain
  • Antonio García-Martín

    • Instituto de Micro y Nanotecnología IMN-CNM, CSIC, CEI UAM + CSIC, Isaac Newton 8, 28760, Tres Cantos, Madrid, Spain
  • Ivan Schuller

    • University of California, San Diego