Strain-enhanced electronic ordering in La<sub>3</sub>Ni<sub>2</sub>O<sub>7</sub> thin films probed by Coherent X-ray Scattering
ORAL
Abstract
We report coherent soft x-ray scattering (CSX) measurements of epitaxial nickelate La3Ni2O7 thin films to investigate nanoscale magnetic ordering associated with the (0.25, 0.25, L) superlattice peak at the Ni L3 resonance (852 eV) and 100K. Using grazing and near-normal-incidence scattering geometries we observe presence of a resonant magnetic Bragg peak. Quantitative analysis of Lorentzian line shapes yields in-plane and out-of-plane correlation lengths of approximately 77 nm and 26 nm, respectively. Fixed-Q energy scans exhibit a pronounced resonance at the Ni L₃ edge, confirming the electronic origin of the modulation. Under coherent illumination, speckle patterns observed within the Bragg peak envelope directly reveal the magnetic domain structure. Time-correlation measurements revealed a gradual decay of speckle intensity under continuous exposure and the formation of localized beam induced damage patches. We quantified the speckle dynamics and found a consistent speckle lifetime τ ≈ 15 - 20 s from 20 - 80 K. Our results demonstrate enhanced in-plane correlations on SrTiO3 substrates, electronic resonance behavior, and the stabilization of large, coherent magnetic domains in bilayer nickelates under tensile strain.
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Presenters
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Arpita Mitra
- Brookhaven National Laboratory (BNL)