Imaging Photonic Resonances within an All-Dielectric Metasurface via Photoelectron Emission Microscopy

ORAL

Abstract

Dielectric metasurfaces exploit light-matter interactions and symmetry to manipulate light for next generation optical devices. Here, we use photoelectron emission microscopy (PEEM) to demonstrate near-field, nanoscale imaging of optical resonances within a dielectric metasurface in the visible wavelength range excited by far-field illumination. The metasurface supports two distinct resonances occupying areas of different material thickness, resulting in contrast in photoemission intensity due to the photoelectron inelastic mean free path (IMFP). Through analysis comparing PEEM images to simulations, we determine the IMFP of very low energy (<1 eV) photoelectrons to be ~35 nm (comparable to meta-atom height), highlighting sensitivity of PEEM to the volume. These results demonstrate that photoelectron imaging is suitable for examining light-matter interactions in volume-type (as opposed to surface) photonic modes within dielectric nanophotonic structures.

*Work was supported by US DoE Office of Science (BES 20-017574) and by LDRD program at SNL and was performed in part at CINT (Office of Science user facility). SNL is a multi-mission laboratory managed by NTESS, a subsidiary of Honeywell International Inc., for the DoE NNSA (contract DE-NA0003525). Views expressed in the article do not necessarily represent the views of the US DoE or the US government.

Publication: https://doi.org/10.1002/adpr.70022

Presenters

  • Andrew R Kim

    • Sandia National Laboratories

Authors

  • Andrew R Kim

    • Sandia National Laboratories
  • Chloe F Doiron

    • Sandia National Laboratories
  • Fernando J Vega

    • Purdue University
  • Jaeyeon Yu

    • Sandia National Laboratories
  • Alex M Boehm

    • Los Alamos National Laboratory
  • Joseph P Klesko

    • Sandia National Laboratories
  • Igal Brener

    • Sandia National Laboratories
  • Raktim Sarma

    • Sandia National Laboratories
  • Alexander Cerjan

    • Sandia National Laboratories
  • Taisuke Ohta

    • Sandia National Laboratories