Optical diode effect at telecom wavelengths in a polar magnet

ORAL

Abstract

Magnetoelectric multiferroics such as rare earth manganites host nonreciprocal behavior driven by low symmetry, spin-orbit coupling, and toroidal moments. Incorporating lanthanide ions like Er3+ extends functionality into the hard infrared for telecom purposes although the localized nature of the excitations is anticipated to weaken magnetoelectric coupling and limit the size of any nonreciprocal effect. In this work, we reveal nonreciprocity in the f-manifold crystal field excitations of h-Lu0.9Er0.1MnO3 demonstrating that, contrary to conventional expectations, localized features in the form of rare earth excitations can host strong dichroic effects. In addition to contrast in the highest fields, we demonstrate nonreciprocity at technologically-relevant energy scales - specifically in the E-, S-, and C-bands of the telecom wavelength range - and at low magnetic fields and room temperature. In fact, the low field behavior is consistent with possible S/A-type altermagnetism in this system. These findings provide a significant conceptual advance in understanding localized excitations in rare earth-containing systems and pave the way for entirely new types of telecom applications.

*Research at the University of Tennessee is supported by Condensed Matter Physics, Division of Materials Research, U. S. National Science Foundation (DMR-2226109).  Work at Rutgers is funded by the W. M. Keck foundation grant to the Keck Center for Quantum Magnetism at Rutgers University. The National High Magnetic Field Laboratory is supported by the National Science Foundation Cooperative Agreement DMR-2128556, the State of Florida, and the U.S. Department of Energy. HSK was supported by the Basic Science Research Program through the National Research Foundation of Korea funded by the Ministry of Science and ICT [Grant No. NRF-2020R1C1C1005900, RS-2023-00220471].

Presenters

  • Kevin A Smith

    • University of Tennessee
    • University of Tennessee, Knoxville

Authors

  • Kevin A Smith

    • University of Tennessee
    • University of Tennessee, Knoxville
  • Yanhong Gu

    • University of Tennessee, Knoxville
    • Brookhaven National Laboratory (BNL)
  • Xianghan Xu

    • University of Minnesota, Twin Cities
  • Heung-Sik Kim

    • Kangwon National University
  • Sang-Wook Cheong

    • Rutgers University
  • Scott A Crooker

    • Los Alamos National Laboratory (LANL)
  • Janice L Musfeldt

    • University of Tennessee