Topological Magneto-optical Kerr Effect without Spin-orbit Coupling in Spin-compensated Antiferromagnet

ORAL

Abstract

The magneto-optical Kerr effect (MOKE), the differential reflection of oppositely circularly polarized light, has traditionally been associated with relativistic spin-orbit coupling (SOC), which links a particle’s spin with its orbital motion. In ferromagnets, large MOKE signals arise from the combination of magnetization and SOC, while in certain coplanar antiferromagnets, SOC-induced Berry curvature enables MOKE despite zero net magnetization. Theoretically, large MOKE can also arise in a broader class of magnetic materials with compensated spins, without relying on SOC - for example, in systems exhibiting real-space scalar spin chirality. The experimental verification has remained elusive. Here, we demonstrate such a SOC- and magnetization-free MOKE in the noncoplanar antiferromagnet Co1/3TaS2. Using a Sagnac interferometer microscope, we image domains of scalar spin chirality and their reversal. Our findings establish experimentally a new mechanism for generating large MOKE signals and position chiral spin textures in compensated magnets as a compelling platform for ultrafast, stray-field-immune opto-spintronic applications.

*This project was supported by the NSF award DMR-2419425 and the Gordon and Betty Moore Foundation through Emergent Phenomena in Quantum Systems (EPiQS) Initiative Grant No. GBMF10276.

Presenters

  • Camron Farhang

    • UMD
    • UCI

Authors

  • Camron Farhang

    • UMD
    • UCI
  • Weihang Lu

    • University of California, Irvine
    • Department of Physics and Astronomy, University of California Irvine
  • Kai Du

    • Fudan University
  • Yunpeng Gao

    • NJIT
    • New Jersey Institute of Technology
  • Junjie Yang

    • New Jersey Institute of Technology
  • Sang-Wook Cheong

    • Rutgers University
  • Jing Xia

    • University of California, Irvine