Exciton dynamics in an atomically thin semiconductor controlled by remote ferroelectric domains

ORAL

Abstract

Ferroelectric domains originating from twisted hexagonal boron nitride (t-hBN) offer a new platform for modulating adjacent functional layers. Here, we investigate how the ferroelectric domains in t-hBN influence exciton diffusion and localization in an adjacent atomically thin MoSe2 layer. The ferroelectric potential imposed by the t-hBN substrate induces two distinct excitonic resonances in MoSe2, one-dimensional excitons localized at domain walls and two-dimensional-like excitons trapped within domains. Time-resolved transient reflection microscopy reveals that these excitons exhibit distinct dynamics behaviors. Our findings establish remote moiré potential engineering as a viable route for tailoring exciton dynamics and transport in two-dimensional optoelectronic systems.

*This work is supported by NSF MRSEC DMR-2308817, the Office of Naval Research via grant N000142512069, and the Welch Foundation Chair F-0014.

Presenters

  • Subin Lee

    • University of Texas at Austin

Authors

  • Subin Lee

    • University of Texas at Austin
  • DONGSEOB KIM

    • The University of Texas at Austin
    • University of Texas at Austin
  • Jose M Torres-Lopez

    • University of Texas at Austin
  • Tomer Amit

    • Weizmann Institute of Science
  • Rigo Mayorga-Luna

    • Texas State University
  • Kenji Watanabe

    • National Institute for Materials Science
    • Research Center for Functional Materials, National Institute of Materials Science, 1-1 Namiki Tsukuba, Ibaraki 305-0044, Japan
  • Takashi Taniguchi

    • National Institute for Materials Science
    • Research Center for Materials Nanoarchitectonics, National Institute for Materials Science
    • International Center for Materials Nanoarchitectonics, National Institute of Materials Science, 1-1 Namiki Tsukuba, Ibaraki 305-0044, Japan
    • Research Center for Functional Materials, National Institute of Materials Science, 1-1 Namiki Tsukuba, Ibaraki 305-0044, Japan
  • Junho Choi

    • Los Alamos National Laboratory (LANL)
  • Sivan Refaely-Abramson

    • Weizmann Institute of Science
  • Allan H MacDonald

    • University of Texas at Austin
  • Xiaoqin Elaine Li

    • University of Texas at Austin