Single electron quantum dot in two-dimensional transition metal dichalcogenides

ORAL  · Invited

Abstract

Two-dimensional transition metal dichalcogenides (TMDCs) offer a compelling platform for spin–valley quantum technologies, but realizing quantum dots (QDs) with sufficiently large orbital level spacing remains a key materials–device challenge. Conventional gate designs used in TMDC QDs struggle to confine carriers tightly enough —an issue amplified in systems with large effective masses such as TMDCs and silicon. In this work, we introduce a multilayer electrostatic architecture that overcomes these constraints and enables the formation of gate-defined TMDC QDs with substantially enhanced energy level separation. Using realistic device modeling, we map how dot size, gate geometry, and dielectric thickness jointly determine the achievable confinement energy. All parameters employed are within current experimental capabilities, offering clear guidance for near-term implementation. This architecture provides a practical route toward achieving spin–valley-resolved quantum states in TMDC QDs and establishes a scalable framework for advancing 2D-material-based quantum devices.

*This research was supported in part by PL-Grid Infrastructure and the Wroclaw Center for Networking and Supercomputing (WCSS). J P acknowledges support from National Science Centre, Poland, under Grant No. 2021/43/D/ST3/01989. This research is supported in part by the Ministry of Education, Singapore, under its Research Centre of Excellence award to the Institute for Functional Intelligent Materials (I-FIM, Project No. EDUNC-33-18-279-V12). K S N is grateful to the Royal Society (UK, Grant Number RSRP\R\190000) for support. K W and T T acknowledge the support from JSPS KAKENHI (Grant Numbers 19H05790, 20H00354 and 21H05233). D.K.P. is grateful to the Agency for Science, Technology, and Research (ASTAR) for support under its ASTAR Career Development Fund (Grant Number C210112039) and the MonArk NSF Quantum Foundry supported by the National Science Foundation Q-AMASE-i program under NSF Award No. DMR-1906383. H.C. acknowledges support from AFOSR Award No. FA9550-19-S-0003.

Publication: https://iopscience.iop.org/article/10.1088/1361-6528/adc81a#artAbst

Presenters

  • Dharmraj Kotekar Patil

    • University of Arkansas

Authors

  • Dharmraj Kotekar Patil

    • University of Arkansas
  • Jarosław Pawłowski

    • Institute of Theoretical Physics, Wrocław University of Science and Technology
  • Pankaj Kumar

    • Institute for Functional Intelligent Materials, National University of Singapore, Singapore
  • Kenji Watanabe

    • National Institute for Materials Science
    • Research Center for Functional Materials, National Institute of Materials Science, 1-1 Namiki Tsukuba, Ibaraki 305-0044, Japan
  • Takashi Taniguchi

    • National Institute for Materials Science
    • Research Center for Materials Nanoarchitectonics, National Institute for Materials Science
    • International Center for Materials Nanoarchitectonics, National Institute of Materials Science, 1-1 Namiki Tsukuba, Ibaraki 305-0044, Japan
    • Research Center for Functional Materials, National Institute of Materials Science, 1-1 Namiki Tsukuba, Ibaraki 305-0044, Japan
  • Kostya S Novoselov

    • Institute for Functional Intelligent Materials, National University of Singapore, Singapore
    • National University of Singapore
  • Hugh Churchill

    • University of Arkansas