Wannier states and spin supersolid physics in a triangular-lattice XXZ antiferromagnet near Ising limit

ORAL

Abstract

The antiferromagnetic Ising model on a triangular lattice is a paradigmatic example of frustrated magnetism. Its ground state lacks long-range order but exhibits macroscopic degeneracy and a finite zero-point entropy, as first shown by Wannier. Introducing a small transverse exchange interaction lifts the classical degeneracy and stabilizes a novel spin supersolid state. In this talk, we present thermodynamic and high-resolution neutron scattering studies on the pseudospin-1/2 triangular lattice antiferromagnet K2Co(SeO3)2, a rare material realization of an easy-axis XXZ Hamiltonian close to the Ising limit [1]. BKT transitions signaling the onset of Ising and supersolid orders are clearly identified, and the Wannier entropy is experimentally recovered. In the supersolid phase, the magnetic excitation spectrum features a broad continuum, with anomalous roton-like minima at its lower boundary. Alongside gapless Goldstone excitations, a pseudo-Goldstone mode with a tiny gap of 0.06 meV is observed. A second continuum is seen at higher energy, replacing the single-spin-flip excitation in the Ising model. Under applied magnetic fields, the Goldstone and pseudo-Goldstone sectors evolve distinctively, and the continuum gradually transforms into coherent spin waves above a field-induced quantum critical point, where the system enters a 1/3-magnetization pletaeu state. These experimental observations show excellent quantitative agreement with quantum Monte Carlo simulations [2].

Publication: [1] M. Zhu, V. Romerio, N. Steiger, S. D. Nabi, N. Murai, S. Ohira-Kawamura, K. Yu. Povarov, Y. Skourski, R. Sibille, L. Keller, Z. Yan, S. Gvasaliya, A. Zheludev, Phys. Rev. Lett. 133, 186704 (2024).
[2] M. Zhu*, Leandro M. Chinellato*, V. Romerio, N. Murai, S. Ohira-Kawamura, Christian Balz, Z. Yan, S. Gvasaliya, Yasuyuki Kato, C. D. Batista, A. Zheludev, npj Quantum Materials 10, 74, (2025).

Presenters

  • Mengze Zhu

    • ETH Zurich

Authors

  • Mengze Zhu

    • ETH Zurich
  • Leandro M Chinellato

    • University of Tennessee
  • Viola F Romerio

    • ETH Zurich
  • Naoki Murai

    • Japan Atomic Energy Agency
  • Seiko O Ohira-Kawamura

    • -PARC Center, Japan Atomic Energy Agency
    • Japan Atomic Energy Agency
    • J-PARC
  • Christian Balz

    • Oak Ridge National Lab
  • Zewu Yan

    • ETH Zurich
    • ETHZ
    • ETH Zürich
  • Severian Gvasaliya

    • ETH Zurich
    • ETHZ
    • ETH Zürich
  • Yasuyuki Kato

    • Univ of Tokyo
  • Cristian D Batista

    • University of Tennessee
  • Andrey Zheludev

    • ETH Zurich