Superconductivity in Ruddlesden-Popper nickel oxides

Oral-In-person

Abstract

In 2023, superconductivity was, for the first time, observed in bulk Ruddlesden-Popper nickelates, in a compressed lanthanum-bearing nickel oxide. Different La-containing nickelate stoichiometries were soon after shown to also superconduct, followed by multiple reports of superconductivity in Pr4Ni3O10 under static pressure. However, this critical phenomenon remains to be explored in nickel alloys grown with elements further down the lanthanide series. The decrease of ionic radius as a function of increasing Z in lanthanides presents another way of tuning the lattice, which could correlate with the pressure threshold needed to drive Ruddlesden-Popper nickelates into a bulk superconducting state.

Publication: X. Chen, E.H.T. Poldi, S. Huyan, R. Chapai, H. Zheng, S.L. Bud'ko, U. Welp, P.C. Canfield, R.J. Hemley, J.F. Mitchell and D. Phelan. "Low fractional volume superconductivity in Pr4Ni3O10 single crystals under pressure". Phys. Rev. B. 111, 094525 (2025).

Presenters

  • Eduardo Poldi

    • University of Illinois at Chicago

Authors

  • Eduardo Poldi

    • University of Illinois at Chicago
  • Xinglong Chen

    • Argonne National Laboratory
  • Hong Zheng

    • Argonne National Laboratory
  • Ulrich Welp

    • Argonne National Laboratory
  • Russell Hemley

    • University of Illinois at Chicago
  • John Mitchell

    • Argonne National Laboratory
  • Daniel Phelan