Quasiparticle description of angle-resolved photoemission spectroscopy for SrCuO2

POSTER

Abstract

Using a high-fidelity diagrammatic many-body theory we show that ARPES in SrCuO2 can be understood as a one-body effect arising from mild disorder in a long-range antiferromagnetic ground state. the emergence of the so-called spinon branch arises naturally from spin disorder, the anomalous linewidths are accurately captured, and we provide a compelling explanation for the spectral weight observed at the non-magnetic zone boundary. This reinterpretation provides a unified explanation for key experimental signatures previously attributed to spin-charge separation, including features observed in optical conductivity. By comparing the spectral features of SrCuO2 with those of La2CuO4, we argue that SrCuO2 shares notable similarities with the two-dimensional cuprates—both being rooted in a common CuO4 plaquette-based molecular orbital framework.

*This work was authored by the National Renewable Energy Laboratory, operated by Alliance for Sustainable Energy, LLC, for the U.S. Department of Energy (DOE) under Contract No. DE-AC36-08 GO28308, funding from Office of Science, Basic Energy Sciences, Division of Materials.

Publication: Dimitar Pashov, Casey Eichstaedt, Swagata Acharya, Mark van Schilfgaarde,
Quasiparticle description of angle-resolved photoemission spectroscopy for SrCuO2,
Computational Materials Today,
Volume 8,
2025,
100041,
ISSN 2950-4635,
https://doi.org/10.1016/j.commt.2025.100041.

Presenters

  • Swagata Acharya

    • National Renewable Energy Laboratory (NREL)
    • National Laboratory of the Rockies

Authors

  • Swagata Acharya

    • National Renewable Energy Laboratory (NREL)
    • National Laboratory of the Rockies