Long-range entanglement and quantum correlations in a multi-frequency comb system

Frequency combs are multimode photonic systems that underlie countless precision sensing and metrology applications. Since their invention over two decades ago, numerous efforts have pushed frequency combs to broader bandwidths and more stable operation. More recently, quantum squeezing and entanglement have been explored in single frequency comb systems for quantum advantages in sensing and signal multiplexing. However, the production of quantum light across multiple frequency combs remains unexplored. In this work, we theoretically explore a mechanism that generates a series of nonlinearly coupled frequency combs through cascaded three-wave upconversion and downconversion processes mediated by a single idler comb. We show how this system generates inter- and intracomb two-mode squeezing and entanglement spanning a very large spectral range, from ultraviolet to mid-IR frequencies. Finally, we show how this system can be engineered to produce on-demand multimode quantum light through covariance matrix optimization. Our findings could enable tunable broadband "ghost" spectroscopy protocols, squeezing-enhanced pump-probe measurements, and broadband entanglement between spectrally-multiplexed quanta of information.