Engineered electron crystals in monolayer MoSe<sub>2</sub> via nano-scale gate patterning

ORAL

Abstract

In two-dimensional electron systems at low temperatures, electrons can organize into a crystalline state known as a Wigner crystal. Wigner crystals have recently been reported in twisted transition metal dichalcogenide semiconductors where a periodic moiré potential is used to further stabilize the crystal. These generalized Wigner crystals are often still constricted by the fixed triangular geometry of moiré potentials. In our work, we take an alternative approach where a lattice is etched into an integrated graphene gate to create a customizable periodic electronic potential. By etching ~ 40 nm triangular lattices into the top gates of an MoSe2 heterostructure, we enable a gate-tunable periodic potential and observe evidence of generalized Wigner crystals at near record high charge densities and temperatures of 2Χ1012 cm-2 and T = 15 K respectively. The integration of a customizable gate opens pathways to engineer previously unattainable programmable quantum states.

*We acknowledge support from NSF Grant Nos. ECCS-2054572, ECCS-2428575, No. ECCS-2122462, ECCS-2235276, AFOSR Grant Nos. FA9550-22-1-0220, FA9550-22-1-0312, FA9550-22-1-0113. This work was additionally supported by the JSPS KAKENHI (Grant Numbers 21H05233 and 23H02052), the CREST (JPMJCR24A5), JST and World Premier International Research Center Initiative (WPI), MEXT, Japan, the Gordon and Betty Moore Foundation grants DOI 10.37807/GBMF13840 and their EPiQS Initiative grant GBMF9069, and the 2023 Technology Research Initiative Fund - National Security Systems - Novel Materials Project, administered by the University of Arizona Office of Research and Partnerships (ORP), funded under Proposition 301, the Arizona Sales Tax for Education Act, in 2000.

Publication: Title: Crystallizing electrons with artificially patterned lattices

Presenters

  • Trevor Stanfill

    • University of Arizona

Authors

  • Trevor Stanfill

    • University of Arizona
  • John R Schaibley

    • University of Arizona
  • Brian J LeRoy

    • University of Arizona
  • Vasili Perebeinos

    • State Univ of NY - Buffalo
  • Takashi Taniguchi

    • National Institute for Materials Science
    • Research Center for Materials Nanoarchitectonics, National Institute for Materials Science
    • International Center for Materials Nanoarchitectonics, National Institute of Materials Science, 1-1 Namiki Tsukuba, Ibaraki 305-0044, Japan
    • Research Center for Functional Materials, National Institute of Materials Science, 1-1 Namiki Tsukuba, Ibaraki 305-0044, Japan
  • Kenji Watanabe

    • National Institute for Materials Science
    • Research Center for Functional Materials, National Institute of Materials Science, 1-1 Namiki Tsukuba, Ibaraki 305-0044, Japan
  • David Mandrus

    • University of Tennessee
  • Michael Koehler

    • University of Tennessee
  • Daniel Noah Shanks

    • NASA Jet Propulsion Laboratory (JPL)