Anisotropic Metallic Electronic Structure of Pd<sub>7</sub><sub>-x</sub>SnTe<sub>2</sub>

ORAL

Abstract

Pd7-xSnTe2 is a layered intermetallic compound exhibiting metallic behavior with a highly anisotropic electronic structure. Angle-resolved photoemission spectroscopy (ARPES) reveals electron-like Fermi surface pockets centered at the M points and weaker hole-like features at Γ, arising from steep dispersive bands without evidence of flat bands or Dirac-like crossings. Polarization-dependent measurements suggest orbital selectivity between Pd d and Te p states but confirm a conventional metallic band topology. In contrast, Pd5AlI2 exhibits orbital-driven frustrated hopping, producing Dirac-like and nearly flat bands characteristic of decorated checkerboard lattices. The comparison establishes Pd7-xSnTe2 as a benchmark anisotropic metal, while Pd₅AlI₂ demonstrates how orbital frustration can drive electronic reconstruction toward correlated or topologically enriched phases. This distinction clarifies how orbital interactions governs the emergence or absence of exotic quantum behaviors in layered intermetallics.

*DOE Office of Science by Brookhaven National Laboratory

Presenters

  • Anjana Krishnadas

    • Brookhaven National Laboratory

Authors

  • Anjana Krishnadas

    • Brookhaven National Laboratory
  • Harshitra Mahalingam

    • Department of Physics, Columbia University, New York, NY, USA
    • Columbia University
  • Vinicius da Silveira Lan Avelar3

    • Department of Chemistry, Columbia University, New York, NY, USA
  • Asish Kundu

    • Brookhaven National Laboratory (BNL)
  • Daniel G Chica

    • Columbia University
    • Department of Chemistry, Columbia University, New York, NY, USA
  • Anil Kumar Rajapitamahuni

    • National Synchrotron Light Source II, Brookhaven National Laboratory, Upton, New York, USA
    • Brookhaven National Laboratory
  • Elio Vescovo

    • Brookhaven National Laboratory
    • National Synchrotron Light Source II, Brookhaven National Laboratory, Upton, New York, USA
  • Raquel Queiroz

    • Department of Physics, Columbia University, New York, NY, USA
    • Columbia University
  • Xavier Roy

    • Columbia University
  • Abhay Pasupathy

    • Columbia University
    • Columbia University/Brookhaven National Laboratory