Magnetic Field-Enhanced Graphene Superconductivity with Record Pauli-Limit Violation

Spin-polarized superconductors offer a rare platform for studying electronic correlations and potentially host non-Abelian quasi-particles, but few candidate systems have been experimentally confirmed to date. Here, we report the observation of a spin-polarized superconducting state, denoted SC5, in WSe₂-proximitized rhombohedral trilayer graphene. At in-plane magnetic field B_|| = 0 T, SC5 has a critical temperature of 68 mK and an out-of-plane critical magnetic field of only 12 mT. Surprisingly, these values are significantly enhanced as B_|| increases, and the superconductivity persists to B_|| = 8.8 T. This value corresponds to a record-high Pauli-limit violation ratio (PVR) of at least 80 among all superconductors, while the true critical field is beyond the limit of our instrument. We conclude that SC5 experiences a canting crossover from Ising-type to spin-polarized superconductor with increased B_||.