Observation of a hidden charge density wave liquid
ORAL
Abstract
Charge density waves (CDWs), electronic crystals that form within a host solid, have long been theorized to melt into a spatially textured electronic liquid. Although such liquid CDWs have not been previously observed, they may be central to the phase diagrams of correlated electron systems, including high temperature superconductors and quantum Hall states. In 1T-TaS2, a promising material for hosting a liquid CDW, a structural phase transition hinders observation. Here, we use femtosecond light pulses to bypass this transition, revealing how topological defect dynamics govern hidden CDW correlations. Following photoexcitation, CDW diffraction peaks broaden azimuthally, indicating the emergence of a hexatic state. At elevated temperatures, photoexcitation fully destroys both translational and orientational order, leaving only a ring of diffuse scattering—a hallmark of a liquid CDW. These findings offer compelling evidence for a defect-unbinding transition to a CDW liquid. More broadly, this approach demonstrates a route to uncover electronic phases obscured by intervening transitions in thermal equilibrium.
*We acknowledge support from the US Department of Energy, Office of Science, Office of Basic Energy Sciences under award no. DE-SC0023017. We also acknowledge support from STROBE: a National Science Foundation Science and Technology Center under Grant No. DMR-1548924.
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Publication: Lee, J.S.H.; Sutter, T.M.; Karapetrov, G.; Musumeci, P.; Kogar, A. Topological Phase Transition to a Hidden Charge Density Wave Liquid. arXiv 2025, arXiv:2505.04867
Presenters
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Joshua Sungho Lee
- University of California, Los Angeles