Interaction of Magnetic Fields with Spinons in a Fractionalized State

ORAL

Abstract

The 4d-electron trimer lattice Ba₄Nb₁₋ₓRu₃₊ₓO₁₂ exhibits either a quantum spin liquid (QSL) or a heavy-fermion strange metal (HFSM) phase, depending on Nb content. In the QSL state, itinerant spinons act as effective heat carriers, enhancing thermal conductivity [1]. Strikingly, applying a magnetic field up to 14 T causes an abrupt, up-to-5000% increase in heat capacity below 150 mK, disrupting the linear temperature dependence typical of both phases. Meanwhile, AC susceptibility and electrical resistivity remain nearly unchanged, while thermal conductivity drops by up to 40% below 4 K. These results suggest spinons, despite being charge-neutral, are highly sensitive to magnetic fields at low temperatures. We propose that the magnetic field could induce Anderson localization of spinons, creating emergent non-magnetic two-level systems responsible for the Schottky-like anomaly in heat capacity. These findings point to a previously unexplored regime of spinon dynamics, potentially governed by field-induced localization and distinct from conventional magnetic or transport signatures [2].

*This work was supported by National Science Foundation via Grant No. DMR 2204811.

Publication: [1] Hengdi Zhao, Yu Zhang, Pedro Schlottmann, Rahul Nandkishore and Gang Cao, Phys. Rev. Lett. 132, 226503 (2024)
[2] Yu Zhang, Hengdi Zhao, Tristan R. Cao, Rahul Nandkishore, Pedro Schlottmann, Lance DeLong and Gang Cao, npj Quantum Materials 10, 86 (2025)

Presenters

  • Gang Cao

    • University of Colorado, Boulder

Authors

  • Gang Cao

    • University of Colorado, Boulder
  • Yu Zhang

    • Argonne National Lab
    • University of Colorado, Boulder
    • Argonne National Laboratory
  • Hengdi Zhao

    • Argonne National Laboratory
    • University of Colorado at Boulder
    • Univeristy of Colorado at Boulder
  • Tristan Cao

    • University of Colorado at Boulder
  • Gabriel Schebel

    • University of Colorado, Boulder
  • Arabella Quane

    • University of Colorado, Boulder
  • Rahul Nandkishore

    • University of Colorado, Boulder
  • Pedro Schlottmann

    • Florida State University
  • Lance Eric De Long

    • University of Kentucky