Exploring Spin Dynamics in One-Dimensional Spin Chains under Driven Conditions

ORAL

Abstract

One-dimensional (1D) quantum spin chains realized in quasi–1D magnets provide an ideal platform to probe entangled many-body dynamics. We investigate their spin dynamics under local energy-absorbing drives that mimic site-selective excitations and quantify their impact on the dynamical spin-structure factor S(q, ω), measurable via inelastic neutron scattering (INS). Using numerically exact time-evolution simulations on large chains, we track the emergence, broadening, and momentum-selective shifts of the S(q, ω) continua, identifying drive-induced pathways that amplify multi-spin-flip correlations and relax the restrictive INS selection rules. We further relate these driven responses to multi–spin-flip excitations observed in resonant inelastic X-ray scattering (RIXS) on chain compounds, clarifying when equilibrium RIXS intensities can serve as a proxy for driven spin dynamics. Our results provide testable predictions for spectral shifts and broadenings in S(q, ω), drive-strength-dependent thresholds, and drive-specific enhancements that can guide future RIXS and INS experiments on candidate 1D magnets.

*This work was supported by the U.S. Department of Energy, Office of Science, Office of Advanced Scientific Computing Research and Office of Basic Energy Sciences, Scientific Discovery through Advanced Computing (SciDAC) program under the CON-NEQT project

Presenters

  • Umesh Kumar

    • Oak Ridge National Laboratory
    • Rutgers University

Authors

  • Umesh Kumar

    • Oak Ridge National Laboratory
    • Rutgers University
  • Gonzalo Alvarez

    • Oak Ridge National Laboratory
  • Satoshi Okamoto

    • Oak Ridge National Laboratory
    • Materials Science and Technology Division, Oak Ridge National Laboratory, Oak Ridge, Tennessee 37831, USA