Photoluminescence as a table top probe of Altermagnetism in the Lieb-Lattice La<sub>2</sub>O<sub>3</sub>Mn<sub>2</sub>Se<sub>2</sub>

ORAL  · Invited

Abstract

Altermagnetism opens a new route to correlated states that couple lattice and spin symmetries, but direct tabletop probes of the Altermagnetic (AM) state remain elusive. Here, I will discuss our efforts to fill this gap by exploring the optical response of La2O3Mn2Se2. This compound was recently reported to host a Mott-insulating AM state on the Lieb lattice, though direct evidence of such a state is elusive. First, I will discuss the optical absorption and photoluminescence (PL) measurements, which combined with the first-principles calculations demonstrate that La2O3Mn2Se2 is a charge-transfer insulator with a strong on-site Hubbard interaction. Furthermore, temperature, excitation energy, and power dependent PL measurements, together with neutron scattering, prove it is magnon-mediated emission from a spin-forbidden (dark) state, both direct consequences of the Altermagnetism.

*The work was supported by the grant DE-SC0018675 funded by the U.S. Department of Energy, Office of Science.

Presenters

  • Kenneth Stephen Burch

    • Boston College

Authors

  • Kenneth Stephen Burch

    • Boston College