Overcoming Epitaxial Constraints through Freestanding Oxide Membranes

Oral-In-person  · Withdrawn

Abstract

Oxide materials display a wide range of functional properties, including ferroelectricity, magnetism, and superconductivity, making them key candidates for next-generation electronic and quantum devices. However, their integration and tunability are often limited by the constraints of epitaxial growth and rigid substrate bonding. Recent advances in freestanding thin-film and membrane techniques enable oxide layers to be detached and transferred onto various substrates, offering new degrees of freedom in material design.

This study explores the use of such transferable oxide membranes to overcome conventional epitaxial limitations and expand the scope of heterostructure engineering. By combining membrane techniques and precise treatments, we reveal how structural reorganization and interface engineering can yield high-quality heterostructures beyond the reach of traditional growth methods. These developments open new directions for oxide heterostructures and device fabrication, transforming how functional materials are combined and integrated.

Publication: Y.-J. Wu, M. Hack, K. Wurster, S. Koch, R. Kleiner, D. Koelle, J. Mannhart, and V. Harbola. Vector-Substrate-Based Josephson Junctions. Appl. Phys. Lett. 125, 032601 (2024).
V. Harbola*, Y.-J. Wu*, F.V.E. Hensling, H. Wang, P.A. van Aken, and J. Mannhart. Vector Substrates: Idea, Design, and Realization. Adv. Funct. Mater. 34, 2306289 (2024).
H. Wang, V. Harbola, Y.-J. Wu, P.A. van Aken, and J. Mannhart. Interface Design Beyond Epitaxy: Oxide
Heterostructures Comprising Symmetry-Forbidden Interfaces. Advanced Materials, 2405065 (2024).

Presenters

  • Yu-Jung Wu

    • Max Planck Institute for Solid State Research

Authors

  • Yu-Jung Wu

    • Max Planck Institute for Solid State Research
  • Varun Harbola

    • Max Planck Institute for Solid State Research
  • Martin Hack

  • Katja Isabelle Wurster

  • Simon Koch

  • Felix Hensling

    • Max Planck Institute for Solid State Physics
  • Hongguang Wang

  • Peter A. van Aken

  • Reinhold Kleiner

    • University of Tuebingen
  • Dieter Koelle

  • Jochen Mannhart

    • Max Planck Institute for Solid State Research