Capacitance measurements of chargons in the spin-liquid candidate YCu<sub>3</sub>(OH)<sub>6</sub>Br<sub>2</sub>[Br<sub>1−y</sub>(OH)<sub>y</sub>] using pulsed magnetic fields of up to 73 T and temperatures down to 0.5 K
ORAL
Abstract
The observation of de Haas-van Alphen-type oscillations in YCOB (YCu3(OH)6Br2[Br1−y(OH)y]), a kagome-lattice Mott insulator with a 3-eV charge gap, has attracted a great deal of attention. The oscillations provide strong evidence for fermionic spinons in a spin liquid that exists near the 1/9 magnetization plateau. An important contribution to this effect is an effective gauge field; even though the spinon is charge neutral, its motion is accompanied by a backflow of orbital chargon current, which couples to the external magnetic field. In order to study the chargons in more detail, we have performed capacitance measurements on YCOB single crystals in pulsed magnetic fields of up to 73 T and at temperatures down to 500 mK. The field range enables capacitance features close to the 1/9 magnetization plateau to be compared directly with those around the 1/3 plateau, which has a different origin. The talk will describe the methods used for sensitive capacitance measurements in the extreme environment of pulsed magnetic fields and show how the features in the capacitance data reflect the underlying spinon statistics.
*The National High Magnetic Field Laboratory (NHMFL) is supported by NSF Cooperative Agreement Nos. DMR-1644779 and DMR-2128556 and the Department of Energy (DOE). J.S. acknowledges support from the DOE BES program "Science at 100 T". Work at the University of Michigan is supported by Department of Energy Award No. DE-SC0020184; Gordon and Betty Moore Foundation Grant No. GBMF5305; and DOE office of Basic Sciences Grant No. DE-FG02-03ER460. Crystal growth was supported by National Key Research and Development Program of China (Grants 2022YFA1403400, No. 2021YFA1400401), the K. C. Wong Education Foundation (Grants No. GJTD-2020-01), and the Strategic Priority Research Program (B) of the Chinese Academy of Sciences (Grants No. XDB33000000).
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Presenters
John Singleton
NHMFL / LANL
Los Alamos National Laboratory (LANL)
Authors
John Singleton
NHMFL / LANL
Los Alamos National Laboratory (LANL)
Noah West
University of Michigan
Kaila G Jenkins
University of Michigan
Guoxin Zheng
California Institute of Technology
Yuan Zhu
University of Michigan
Dechen Zhang
University of Michigan
Shiliang Li
Institute of Physics, Chinese Academy of Sciences
Beijing National Laboratory for Condensed Matter Physics, Institute of Physics, Chinese Academy of Sciences, Beijing 100190, China