Pump Wavelength Dependent Time Correlated Photoluminescence Spectroscopy of Giant Quantum Dots

POSTER

Abstract

Quantum dots have gained significance as high quantum yield photon sources in many applications. A new breed of ``giant'' quantum dots (gQDs) developed at Los Alamos National Labs consisting of a CdSe core coated with several mono-layers of CdS have shown suppressed blinking [1]. gQDs have been shown to exhibit two types of blinking -- Type A, associated with short off-state lifetime and Type B, characterized by long off-state lifetime [2]. However, the appearance of A or B type blinking is unpredictable and intermittent. We conduct pump wavelength dependent time correlated PL spectroscopy on gQDs to narrow down the causes of appearance of these blinking types. Our results suggest that there is a faster PL decay when excitons are pumped in the shell as compared to when only the core is pumped. This suggests that pumping the core opens up various non radiative decay channels, some of which may lead to type B blinking. Studies on dependence of blinking rates on pump wavelength are currently undergoing. \\[4pt] [1] Malko et al; Pump Intensity and Shell Thickness Dependent Evolution of Photoluminescence Blinking in Individual Core/Shell CdSe/CdS Nanocrystals; nl2025272 \\[0pt] [2] Galland \textit{et al}; Two types of luminescence blinking revealed by spectroelectrochemistry of single quantum dots; nature10569

Authors

  • Aalap Verma

    University of Texas at Dallas

  • Siddharth Sampat

    University of Texas at Dallas

  • Anton Malko

    University of Texas at Dallas

  • Iman Rezanejad

    TAMU, TTU, TCU, Texas State University, Department of Physics, Texas Tech University, Lubbock, TX, Department of Chemistry \& Biochemistry, Texas Tech University, Lubbock, TX, Department of Mechanical Engineering, Texas Tech University, Lubbock, TX, Universidade de Sao Paulo, Ohio University, Stanford University, University of Waterloo, Canada, Institute for Quantum Science and Engineering (IQSE) and Department of Physics and Astronomy, Texas A\&M University, Beijing Computational Science Research Center, Beijing, China, Institute for Quantum Studies and Department of Physics, Texas A\&M University, College Station, Texas 77843, USA, Texas A\&M University at Qatar, Education City, P.O. Box 23874, Doha, Qatar, TTU Center for Pulsed Power and Power Electronics, Texas A\&M University - Commerce, Meyer Observatory, Clifton TX, CASPER, Baylor University, Waco TX, CASPER NSF-REU, Baylor University, Waco TX, Texas Tech University, University of Texas at Dallas, Oklahoma University, Princeton University, University of Chicago, Cornell University, Los Alamos National Laboratory, Department of Physics, Lamar University, Department of Physics \& Geosciences, Angelo State University, Brookhaven National Laboratory, Fermi National Accelerator Laboratory, Texas A\&M University, Physics Dept, Texas State University, San Marcos, Istanbul University, Department of Electrical Engineering, University of Texas at Arlington, Department of Physics \& Astronomy, University of Texas at Brownsville, V. N. Bakul Institute for Superhard Materials, University of North Texas, Department of Physics, TCU, Department of Physics and Astronomy, Department of Computer Science, Texas State University at San Marcos, Department of Physics, Texas State University at San Marcos, Institute for Quantum Science and Engineering and Department of Physics and Astronomy, Texas A\&M University, College Station, Texas 77843, USA, The National Center for Mathematics and Physics, KACST, P.O. Box 6086, Riyadh 11442, Saudi Arabia, Key Laboratory of Quantum Information, University of Science and Technology of China, Hefei, Anhui, 230026, People's Republic of China, Department of Physics, the University of Texas at Dallas, Richardson, TX, 75080 USA, State Key Laboratory of Quantum Optics and Quantum Optics Devices, College of Physics and Electronic Engineering, Shanxi University, Taiyuan 030006, Department of Physics and Astronomy, Washington State University, Pullman, Washington, 99164 USA, University of Guelph, Guelph Canada, Department of Physics, National Chung Cheng University, Chia-Yi 621, Taiwan, University of Houston Clear Lake, The University of Texas at Dallas, The University of Texas at San Antonio, Angelo State University, Department of Physics and Astronomy and Center for Gravitational Wave Astronomy, University of Texas at Brownsville, Brownsville, Texas 78520 USA, Laboratoire des Mat\'eriaux Avanc\'es, Universit\'e Claude Bernard Lyon 1, Campus de la DOUA, Villeurbanne Cedex 69622 France, Department of Engineering, University of Texas at Brownsville, Brownsville, Texas 78520 USA, BAE Systems, Advanced Systems and Technology, Nashua, NH, Istanbul University, Beyazit 3449 Istanbul, Turkey, Texas Tech University, Physics, Texas Tech University, Lubbock, TX, Istanbul University, Istanbul, Turkey, Arkansas State University, Jonesboro, AK, Abilene Christian University, Department of Physics and Astronomy, Clemson University, Clemson, SC, 29634 USA, Department of Physics, University of Texas at El Paso, Qatar Biomedical Research Institute, Texas A\&M University at Qatar, FUTY, Yola, Adamawa State, Nigeria, FUTY, Yola, Adamawa State, Department of Physics, University of Abuja, Abuja, Nigeria, Department of Electrical and Computer Engineering, Texas A\&M University

  • Iman Rezanejad

    TAMU, TTU, TCU, Texas State University, Department of Physics, Texas Tech University, Lubbock, TX, Department of Chemistry \& Biochemistry, Texas Tech University, Lubbock, TX, Department of Mechanical Engineering, Texas Tech University, Lubbock, TX, Universidade de Sao Paulo, Ohio University, Stanford University, University of Waterloo, Canada, Institute for Quantum Science and Engineering (IQSE) and Department of Physics and Astronomy, Texas A\&M University, Beijing Computational Science Research Center, Beijing, China, Institute for Quantum Studies and Department of Physics, Texas A\&M University, College Station, Texas 77843, USA, Texas A\&M University at Qatar, Education City, P.O. Box 23874, Doha, Qatar, TTU Center for Pulsed Power and Power Electronics, Texas A\&M University - Commerce, Meyer Observatory, Clifton TX, CASPER, Baylor University, Waco TX, CASPER NSF-REU, Baylor University, Waco TX, Texas Tech University, University of Texas at Dallas, Oklahoma University, Princeton University, University of Chicago, Cornell University, Los Alamos National Laboratory, Department of Physics, Lamar University, Department of Physics \& Geosciences, Angelo State University, Brookhaven National Laboratory, Fermi National Accelerator Laboratory, Texas A\&M University, Physics Dept, Texas State University, San Marcos, Istanbul University, Department of Electrical Engineering, University of Texas at Arlington, Department of Physics \& Astronomy, University of Texas at Brownsville, V. N. Bakul Institute for Superhard Materials, University of North Texas, Department of Physics, TCU, Department of Physics and Astronomy, Department of Computer Science, Texas State University at San Marcos, Department of Physics, Texas State University at San Marcos, Institute for Quantum Science and Engineering and Department of Physics and Astronomy, Texas A\&M University, College Station, Texas 77843, USA, The National Center for Mathematics and Physics, KACST, P.O. Box 6086, Riyadh 11442, Saudi Arabia, Key Laboratory of Quantum Information, University of Science and Technology of China, Hefei, Anhui, 230026, People's Republic of China, Department of Physics, the University of Texas at Dallas, Richardson, TX, 75080 USA, State Key Laboratory of Quantum Optics and Quantum Optics Devices, College of Physics and Electronic Engineering, Shanxi University, Taiyuan 030006, Department of Physics and Astronomy, Washington State University, Pullman, Washington, 99164 USA, University of Guelph, Guelph Canada, Department of Physics, National Chung Cheng University, Chia-Yi 621, Taiwan, University of Houston Clear Lake, The University of Texas at Dallas, The University of Texas at San Antonio, Angelo State University, Department of Physics and Astronomy and Center for Gravitational Wave Astronomy, University of Texas at Brownsville, Brownsville, Texas 78520 USA, Laboratoire des Mat\'eriaux Avanc\'es, Universit\'e Claude Bernard Lyon 1, Campus de la DOUA, Villeurbanne Cedex 69622 France, Department of Engineering, University of Texas at Brownsville, Brownsville, Texas 78520 USA, BAE Systems, Advanced Systems and Technology, Nashua, NH, Istanbul University, Beyazit 3449 Istanbul, Turkey, Texas Tech University, Physics, Texas Tech University, Lubbock, TX, Istanbul University, Istanbul, Turkey, Arkansas State University, Jonesboro, AK, Abilene Christian University, Department of Physics and Astronomy, Clemson University, Clemson, SC, 29634 USA, Department of Physics, University of Texas at El Paso, Qatar Biomedical Research Institute, Texas A\&M University at Qatar, FUTY, Yola, Adamawa State, Nigeria, FUTY, Yola, Adamawa State, Department of Physics, University of Abuja, Abuja, Nigeria, Department of Electrical and Computer Engineering, Texas A\&M University

  • Iman Rezanejad

    TAMU, TTU, TCU, Texas State University, Department of Physics, Texas Tech University, Lubbock, TX, Department of Chemistry \& Biochemistry, Texas Tech University, Lubbock, TX, Department of Mechanical Engineering, Texas Tech University, Lubbock, TX, Universidade de Sao Paulo, Ohio University, Stanford University, University of Waterloo, Canada, Institute for Quantum Science and Engineering (IQSE) and Department of Physics and Astronomy, Texas A\&M University, Beijing Computational Science Research Center, Beijing, China, Institute for Quantum Studies and Department of Physics, Texas A\&M University, College Station, Texas 77843, USA, Texas A\&M University at Qatar, Education City, P.O. Box 23874, Doha, Qatar, TTU Center for Pulsed Power and Power Electronics, Texas A\&M University - Commerce, Meyer Observatory, Clifton TX, CASPER, Baylor University, Waco TX, CASPER NSF-REU, Baylor University, Waco TX, Texas Tech University, University of Texas at Dallas, Oklahoma University, Princeton University, University of Chicago, Cornell University, Los Alamos National Laboratory, Department of Physics, Lamar University, Department of Physics \& Geosciences, Angelo State University, Brookhaven National Laboratory, Fermi National Accelerator Laboratory, Texas A\&M University, Physics Dept, Texas State University, San Marcos, Istanbul University, Department of Electrical Engineering, University of Texas at Arlington, Department of Physics \& Astronomy, University of Texas at Brownsville, V. N. Bakul Institute for Superhard Materials, University of North Texas, Department of Physics, TCU, Department of Physics and Astronomy, Department of Computer Science, Texas State University at San Marcos, Department of Physics, Texas State University at San Marcos, Institute for Quantum Science and Engineering and Department of Physics and Astronomy, Texas A\&M University, College Station, Texas 77843, USA, The National Center for Mathematics and Physics, KACST, P.O. Box 6086, Riyadh 11442, Saudi Arabia, Key Laboratory of Quantum Information, University of Science and Technology of China, Hefei, Anhui, 230026, People's Republic of China, Department of Physics, the University of Texas at Dallas, Richardson, TX, 75080 USA, State Key Laboratory of Quantum Optics and Quantum Optics Devices, College of Physics and Electronic Engineering, Shanxi University, Taiyuan 030006, Department of Physics and Astronomy, Washington State University, Pullman, Washington, 99164 USA, University of Guelph, Guelph Canada, Department of Physics, National Chung Cheng University, Chia-Yi 621, Taiwan, University of Houston Clear Lake, The University of Texas at Dallas, The University of Texas at San Antonio, Angelo State University, Department of Physics and Astronomy and Center for Gravitational Wave Astronomy, University of Texas at Brownsville, Brownsville, Texas 78520 USA, Laboratoire des Mat\'eriaux Avanc\'es, Universit\'e Claude Bernard Lyon 1, Campus de la DOUA, Villeurbanne Cedex 69622 France, Department of Engineering, University of Texas at Brownsville, Brownsville, Texas 78520 USA, BAE Systems, Advanced Systems and Technology, Nashua, NH, Istanbul University, Beyazit 3449 Istanbul, Turkey, Texas Tech University, Physics, Texas Tech University, Lubbock, TX, Istanbul University, Istanbul, Turkey, Arkansas State University, Jonesboro, AK, Abilene Christian University, Department of Physics and Astronomy, Clemson University, Clemson, SC, 29634 USA, Department of Physics, University of Texas at El Paso, Qatar Biomedical Research Institute, Texas A\&M University at Qatar, FUTY, Yola, Adamawa State, Nigeria, FUTY, Yola, Adamawa State, Department of Physics, University of Abuja, Abuja, Nigeria, Department of Electrical and Computer Engineering, Texas A\&M University