Comparison of Monocrystalline Nanocubes and Polycrystalline Nanospheres of Fe3O4

POSTER

Abstract

This report describes synthesis of monocrystalline Fe3O4 nanocubes and polycrystalline nanospheres with tunable body diagonals and diameters via solvothermal and thermal decomposition reactions. The dimensions of the spherical MNPs were tuned to obtain particles for one set of spherical MNPs the volume was equivalent to that of a targeted cubic MNP volume and for a second set of spherical MNPs the diameter was equivalent to the body diagonal of a targeted batch of cubic MNPs. The PPMS was used to compare the magnetic properties of the synthesized spherical and cubic Fe3O4 MNPs on a volume and diameter/body diagonal basis. As compared to polycrystalline nanospheres, there is a higher saturation magnetization for nanocubes, which makes them more attractive for biosensing applications. The synthesized nanocubes also have a significantly higher coercivity as compared to their nanospherical counterparts with the same volume or equivalent diameter. This makes them more suitable for hyperthermia applications in which the heat generated varies linearly with coercivity. With this study, we demonstrate that shape is an important parameter that can be used to manipulate nanoscale magnetism in Fe3O4 MNPs in order to tailor them for a particular application.

Authors

  • Arati Kolhatkar

    University of Houston

  • Chamath Dannangoda

    University of Texas at Brownsville, The University of Texas at Brownsville

  • Hanu Arava

    University of Houston, University of Texas at Brownsville, None, Univ of Texas, San Antonio, University of Texas at El Paso, Univ of Arizona, Department of Physics and Astronomy and Center for Gravitational Wave Astronomy, University of Texas at Brownsville, Laboratoire des Mat\'eriaux Avanc\'es, Universit\'e Claude Bernard Lyon 1, UTEP, University of Texas, Austin, University of Texas at Austin, Institute for Astronomy, Russian Academy of Sciences, University of Texas at Arlington, The University of Texas at Arlington, MIT, U. Mass. Dartmouth, Texas A{\&}M University, Texas Christian University, Laboratoire des Mat\'erieux Avanc\'es B\^atiment Virgo, Ion Beam Materials Laboratory, Los Alamos National Laboratory, Texas A\&M University, Accelerator Research Laboratory, University of Florida, The Ohio State University, Yale University, University of Guelph, Canada, Armagh Observatory, NASA-Ames, NASA-Goddard, Texas A\&M University-Commerce, Texas A\&M University, Hanyang University, Texas A\&M Univ, Department of Pharmacy, Mazandaran University of Medical Sciences, Sari, Iran, Physics Department, Texas State University at San Marcos

  • Hanu Arava

    University of Houston, University of Texas at Brownsville, None, Univ of Texas, San Antonio, University of Texas at El Paso, Univ of Arizona, Department of Physics and Astronomy and Center for Gravitational Wave Astronomy, University of Texas at Brownsville, Laboratoire des Mat\'eriaux Avanc\'es, Universit\'e Claude Bernard Lyon 1, UTEP, University of Texas, Austin, University of Texas at Austin, Institute for Astronomy, Russian Academy of Sciences, University of Texas at Arlington, The University of Texas at Arlington, MIT, U. Mass. Dartmouth, Texas A{\&}M University, Texas Christian University, Laboratoire des Mat\'erieux Avanc\'es B\^atiment Virgo, Ion Beam Materials Laboratory, Los Alamos National Laboratory, Texas A\&M University, Accelerator Research Laboratory, University of Florida, The Ohio State University, Yale University, University of Guelph, Canada, Armagh Observatory, NASA-Ames, NASA-Goddard, Texas A\&M University-Commerce, Texas A\&M University, Hanyang University, Texas A\&M Univ, Department of Pharmacy, Mazandaran University of Medical Sciences, Sari, Iran, Physics Department, Texas State University at San Marcos

  • Hanu Arava

    University of Houston, University of Texas at Brownsville, None, Univ of Texas, San Antonio, University of Texas at El Paso, Univ of Arizona, Department of Physics and Astronomy and Center for Gravitational Wave Astronomy, University of Texas at Brownsville, Laboratoire des Mat\'eriaux Avanc\'es, Universit\'e Claude Bernard Lyon 1, UTEP, University of Texas, Austin, University of Texas at Austin, Institute for Astronomy, Russian Academy of Sciences, University of Texas at Arlington, The University of Texas at Arlington, MIT, U. Mass. Dartmouth, Texas A{\&}M University, Texas Christian University, Laboratoire des Mat\'erieux Avanc\'es B\^atiment Virgo, Ion Beam Materials Laboratory, Los Alamos National Laboratory, Texas A\&M University, Accelerator Research Laboratory, University of Florida, The Ohio State University, Yale University, University of Guelph, Canada, Armagh Observatory, NASA-Ames, NASA-Goddard, Texas A\&M University-Commerce, Texas A\&M University, Hanyang University, Texas A\&M Univ, Department of Pharmacy, Mazandaran University of Medical Sciences, Sari, Iran, Physics Department, Texas State University at San Marcos

  • Hanu Arava

    University of Houston, University of Texas at Brownsville, None, Univ of Texas, San Antonio, University of Texas at El Paso, Univ of Arizona, Department of Physics and Astronomy and Center for Gravitational Wave Astronomy, University of Texas at Brownsville, Laboratoire des Mat\'eriaux Avanc\'es, Universit\'e Claude Bernard Lyon 1, UTEP, University of Texas, Austin, University of Texas at Austin, Institute for Astronomy, Russian Academy of Sciences, University of Texas at Arlington, The University of Texas at Arlington, MIT, U. Mass. Dartmouth, Texas A{\&}M University, Texas Christian University, Laboratoire des Mat\'erieux Avanc\'es B\^atiment Virgo, Ion Beam Materials Laboratory, Los Alamos National Laboratory, Texas A\&M University, Accelerator Research Laboratory, University of Florida, The Ohio State University, Yale University, University of Guelph, Canada, Armagh Observatory, NASA-Ames, NASA-Goddard, Texas A\&M University-Commerce, Texas A\&M University, Hanyang University, Texas A\&M Univ, Department of Pharmacy, Mazandaran University of Medical Sciences, Sari, Iran, Physics Department, Texas State University at San Marcos

  • Hanu Arava

    University of Houston, University of Texas at Brownsville, None, Univ of Texas, San Antonio, University of Texas at El Paso, Univ of Arizona, Department of Physics and Astronomy and Center for Gravitational Wave Astronomy, University of Texas at Brownsville, Laboratoire des Mat\'eriaux Avanc\'es, Universit\'e Claude Bernard Lyon 1, UTEP, University of Texas, Austin, University of Texas at Austin, Institute for Astronomy, Russian Academy of Sciences, University of Texas at Arlington, The University of Texas at Arlington, MIT, U. Mass. Dartmouth, Texas A{\&}M University, Texas Christian University, Laboratoire des Mat\'erieux Avanc\'es B\^atiment Virgo, Ion Beam Materials Laboratory, Los Alamos National Laboratory, Texas A\&M University, Accelerator Research Laboratory, University of Florida, The Ohio State University, Yale University, University of Guelph, Canada, Armagh Observatory, NASA-Ames, NASA-Goddard, Texas A\&M University-Commerce, Texas A\&M University, Hanyang University, Texas A\&M Univ, Department of Pharmacy, Mazandaran University of Medical Sciences, Sari, Iran, Physics Department, Texas State University at San Marcos