Ferromagnetism with Continuum Excitations in the Geometrically Frustrated Pyrochlore Yb$_2$Ti$_2$O$_7$

COFFEE_KLATCH · Invited

Abstract

In the frustrated pyrochlore magnet Yb$_2$Ti$_2$O$_7$, Yb$^{3+}$ forms (effective) S=1/2 moments that are subject to anisotropic exchange interactions. The ground state of this material is rather perplexing and controversial; one proposal is that Yb$_2$Ti$_2$O$_7$ behaves as a quantum version of ``spin ice'', where quantum fluctuations enable tunneling between different ice-rules obeying spin states. This model includes a quantum spin liquid ground state hosting three exotic quasi-particle excitations that are analogs of magnetic monopoles, electric monopoles, and photons; i.e., it would host a full ``emergent electrodynamics''. However, there are varying reports about the true nature of the ground state in Yb$_2$Ti$_2$O$_7$, in part due to a known sample-dependence involving non-stoichiometry on the 1\% level, which is particularly prevalent in single crystal samples. After introducing the key prior measurements on Yb$_2$Ti$_2$O$_7$, I will present neutron scattering results from a polycrystalline sample which is known to be stoichiometric. This sample was found to develop magnetic Bragg peaks at low temperatures, consistent with moments forming a long range ordered ferromagnetic state. Despite this signature of a long range ordered ground state, the spin excitations remain gapless and continuum-like (unlike the expectation for conventional magnons), and are generally insensitive to the first order transition at 260 mK which is observed via specific heat measurements.

Authors

  • Kate Ross

    Colorado State University