Photodetachment dynamics in a strong single-cycle terahertz pulse

POSTER

Abstract

We present theory and calculations for the photodetachment dynamics of negative ions driven by a single-cycle terahertz pulse. The photoelectron can follow two or more classical trajectories to arrive at a detector simultaneously, allowing the electron waves to interfere quantum mechanically. For negative hydrogen and fluorine ions, both the in-phase and antiphase interference oscillations are observed in the temporal electron flux recorded at a large distance (0.5m). As the terahertz pulse gets strong enough, an oscillatory photodetachment rate can be observed, which arises from the quantum interferences near the source region caused by the returning electron waves following three types of closed classical orbits. Our semiclassical formulas are proved to be quantitatively accurate by comparing with exact quantum simulations. The presented theory could also be generalized for other similar systems where the electron experiences an interaction with an applied electric-field driving pulse.

Authors

  • Baochun Yang

    Purdue Univ

  • Francis Robicheaux

    Purdue University, Purdue Univ, Department of Physics and Astronomy, Purdue University, West Lafayette, Indiana 47907, USA