Analysis of multi-orbital contributions in HHG spectra through multiple single active electron simulations

POSTER

Abstract

In multielectron atoms, full ab-initio simulation of high harmonic generation (HHG) spectra is not computationally feasible. The single active electron (SAE) approximation considers the dynamics of one electron in a frozen potential from the remaining electrons. Comparisons with multielectron methods (TDDFT, MCTDHF) have shown that SAE simulations (for an electron in the outer valence shell) often accurately reproduce HHG spectra up to the active electron's cut-off ($I_p+3.17U_p$) but fail to reproduce a second or extended plateau attributed to inner-shell electrons. We present inner-shell SAE potentials and simulations which, in conjunction with valence SAE results, display the expected plateau behavior without dynamic multielectron interactions.

Authors

  • Ran Reiff

    JILA and Department of Physics, University of Colorado, Boulder

  • Tennesse Joyce

    JILA and Department of Physics, University of Colorado, Boulder

  • Agnieszka Jaron-Becker

    JILA and Department of Physics, University of Colorado, Boulder

  • Andreas Becker

    JILA and Department of Physics, University of Colorado, Boulder