KMnF<sub>3</sub> Thin Film Epitaxial Growth and Characterization

Oral-In-person

Abstract

Interest in antiferromagnets (AFMs) as promising materials for modern spintronics and magnonics arises from their ultrafast dynamics, nanoscale integration compatibility, and insensitivity to stray fields [1]. However, several AFMs that have been historically well-characterized in bulk have not been characterized in thin films.

Using molecular beam epitaxy, we grew KMnF3 [2-4] films of varying thickness and crystal quality. Electron diffraction confirms our films are monocrystalline with a high degree of crystallinity. Additionally, X-ray analysis shows the films have a cubic crystal structure at RT with a lattice constant of 4.189Å, which perfectly matches the structure of the bulk. The ongoing magnetic investigation of the KMnF3 reveals a complex band structure very sensitive to temperature. Our studies open the door to applications of epitaxial KMnF3 films for magnonic and spintronic experiments.

[1] J. Han et al., Nature Materials, 22, 684 (2023)

[1] O. Beckman and K. Knox, Phys. Rev. 121, 376 (1961).

[2] A. J. Heeger, O. Beckman, and A. M. Portis, Phys. Rev. 123, 1652 (1961).

[3] K. S. Knight, et al., Journal of Alloys and Compounds 842, 155935 (2020).

Publication: O. G. Zanoni et al. KMnF3 Thin Film Growth by Molecular Beam Epitaxy and Characterization. In preparation.

Presenters

  • Olivia Zanoni

    • University of Colorado, Colorado Springs

Authors

  • Olivia Zanoni

    • University of Colorado, Colorado Springs
  • Dario Bueno-Baques

    • University of Colorado, Colorado Springs
  • Randy Dumas

    • Quantum Design Inc.
  • Yi Li

    • Argonne National Laboratory
  • Valentine Novosad

    • Argonne National Laboratory
  • Zbigniew Celinski

    • University of Colorado, Colorado Springs
  • Dmytro Bozhko

    • University of Colorado Colorado Springs